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Ordered carbonaceous residues appear to form on [9(100) x (loo)]; disordered on [7(111) x (310)], which has a high concentration of kinks in the steps. Pt displays a unique surface chemistry in that low co-ordination number sites on steps and kinks are responsible for bond-breaking processes. Ir differs from Pt in that, even on low-index faces, partial decomposition of hydrocarbons may occur. Pt and perhaps Pd and Ni have the ability to show this variation in activity when one compares low- and high-index faces, where the conditions are low temperature and pressure.

Schachter, Acta Chim. Acad. Sci. , 1968, 58, 321. R. Joyner, J. Catalysis, 1977, 50, 176. - 29 Catalysis on Metal Surfaces and Non-metallic Substrates CH CH I\ I M--M CH-CH I M Thus effectiveness in breaking down CO becomes a pointer to effectiveness in Fischer-Tropsch catalysis. After considering more evidence in favour of his model, Joyner then considers very thoughtfully possible criticisms. The relationship between heat of adsorption of CO and catalytic conversion for CO and H 2 on a wide range of metals is well supported in Vannice’s6’ volcano-shaped curves for CO adsorptions on alumina-supported metals.

Vroom, J . Carafysis, 1977, 50,244. R. D. Kelley, T. E. Madey, and J. T. Yates, J . Catalysis, 1977, 50, 301. J. R. H. Ross in ‘Surface and Defect Properties of Solids’, ed. M. W. Roberts and J. M. Thomas (Specialist Periodical Reports), The Chemical Society, London, 1975, Vol. 4, p. 34. J. R. H. Ross, M. C. F. Steel, and A. Zeine-Isfahani, J . Catalysis, 1978, 52, 280. M. Flytzani-Stephanopoulos, S. Wong, and L. D. Schmidt, J . Catalysis, 1977, 49, 51. F. BOZSO,G. Ertl, M. Grunze, and M. Weiss, J .

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